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Accepted Manuscript - Portal de docentes FCT/UNL
Accepted Manuscript
Title: Electrochemical biosensor based on biomimetic material
for myoglobin detection
Author: Felismina T.C. Moreira Rosa A.F. Dutra João P.C.
Noronha M. Goreti F. Sales
PII:
DOI:
Reference:
S0013-4686(13)01167-5
http://dx.doi.org/doi:10.1016/j.electacta.2013.06.061
EA 20704
To appear in:
Electrochimica Acta
Received date:
Revised date:
Accepted date:
28-3-2013
19-6-2013
21-6-2013
Please cite this article as: F.T.C. Moreira, R.A.F. Dutra, J.P.C. Noronha, M.G.F. Sales,
Electrochemical biosensor based on biomimetic material for myoglobin detection,
Electrochimica Acta (2013), http://dx.doi.org/10.1016/j.electacta.2013.06.061
This is a PDF file of an unedited manuscript that has been accepted for publication.
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Ô
+
¸
¹
¸
î
Ï
Ý
½
¼
½
Í
B
+
ï
À
¿
½
Ý
¼
à
Í
¼
Ï
¼
×
Û
À
Ø
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1
w
;
B
6
'
A
;
!
;
+
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H
;
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!
C
+
|
C
+
+
1
/
z
+
E
=
7
C
7
*
{
x
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(
B
y
C
<
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C
+
B
+
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+
1
1
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B
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!
C
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B
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&
+
1
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1
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B
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H
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1
w
x
5
y
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w
6
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x
y
+
C
1
+
w
;
B
;
B
+
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B
B
+
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C
!
B
1
w
A
V
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š
=
L
1
;
B
+
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H
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1
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A
B
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+
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+
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+
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+
w
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;
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C
+
1
;
w
!
C
1
;
B
+
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*
C
w
H
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$
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A
B
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C
;
!
@
<
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C
B
+
=
1
+
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1
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B
C
w
+
1
;
w
!
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&
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†
—
(
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†
ž
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Ÿ
ž
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+
†
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†
—
)
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#
1
;
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B
C
B
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A
w
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x
7
,
y
/
z
E
7
7
{
H
@
<
B
<
A
w
+
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!
;
+
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|
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N
L
N
T
B

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1
{
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1
B
=
C
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1
w
x
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-
y
=
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,
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1
B
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B
1
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T
V
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L
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1
w
1
A
B
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1
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+
w
A
C
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B
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x
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y
H
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1
K
L
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J
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L
&
B
S
1
K
T
L
C
}
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1
S
J
B

B
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1
H
@
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A
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+
H
1
B
1
+
1
B
B
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&
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A
A
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1
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1
w
B
C
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1
1
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1
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C
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K
V
T
+
M
B
}
L
B
C

;
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H
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+
1
+
1
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B
0
+
+
+
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B
+
1
B
1
<
B
=
%
!
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1
C
+
%
<
9
!

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B
!
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H
H
+
1
+
1
1
w
<
!
U
w
-
x
7
{
y
C
*
B
+
+
1
;
w
!
B
C
H
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*
+
@
<
+
A
w
B
A
=
+
1
/
z
E
7
7
{
<
w
x
y
(
+
A
<
A
=
<
+
/
z
E
7
7
{
&
H
+
1
+
1
U
B
;
+
1
!
+
=
C
B
+
A
<
C
!
w
1
!
=
A
<
B
+
!
<
+
K
K
J
L
B

"
*
=
=
+
<
+
1
B
C
<
=
!
*
;
C
!
+
1
;
!
+
-
x
7
0
-
{
y
,
1
+
H
A
<
+
A
*
+
S
J
M
<
}
S
M
B

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C
!
w
A
*
+
C
+
+
w
&
B
‚
*
B
C
A
=
H
!
B
B
+
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+
+
1
+
1
!
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1
;
w
!
D
+
+
;
x
)
y
;
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+
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=
1
+
+
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1
6
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;
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C
C
+
1
+
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1
)
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!
+
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+
H
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+
=
C
B
+
A
B
*
w
<
C
*
B
+
H
!
+
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B
<
&
A
+
1
A
w
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E
|
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+
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B
+
*
!
&
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+
1
w
H
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w
+
1
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B
=
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1
;
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@
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&
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1
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#
%
%
=
(
$
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%
%
&
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;
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<
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$
$
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$
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+
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H
$
B
;
$
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H
&
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$
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$
$
$
&
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<
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%
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$
+
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+
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;
w
<
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+
A
<
!
K
L
V
J
B

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+
1
+
H
=
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+
-
0
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+
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B
1
=
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+
1
0
+
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1
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A
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B
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<
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A
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+
M
M
M
B

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3
+
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1
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)
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1
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C
!
+
1
;
w
!
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+
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B
+
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&
+
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+
|
w
+
1
+
+
1
+
w
;
B
A
<
C
+
1
+
1
-
.
<
=
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;
H
!
+
C
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+
1
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B
;
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@
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w
/
0
1
2
3
Ô
¸
·
¸
·
¸
þ
×
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à
¾
½
Ö
à
Ü
Í
ß
Ø
à
¼
×
î
ß
»
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ï
¼
Ï
à
Í
Õ
»
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à
¾
½
Ö
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à
Ö
»
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4
5
-
6
-
-
-
.
-
/
-
1
!
<
E
=
+
+
B
;
<
!
A
C
B
+
1
C
B
1
=
=
<
3
B
/
:
A
*
!
C
A
B
!
@
<
U
;
A
B
w
+
<
+
B
+
!
1
=
=
+
1
+
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-
-
5
.
6
!
;
.
-
.
.
.
/
6
+
!
B
*
+
+
1
;
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+
C
B
+
!
B
!
B
C
H
|
H
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U
w
+
&
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B
1
7
8
9
:
;
<
=
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%
>

9
7
8
9
:
;
<
=
$
>

3
@
!
B
+
!
B
1
B
!
1
w
A
*
<
C
!
+
1
;
*
!
;
&
A
=
:
6
3
C
+
1
+
+
@
@
*
+
+
1
B
1
=
!
+
B
C
Randle’s equivalent circuit was adopted
+
+
1
;
<
w
+
1
!
;
*
!
!
B
C
B
+
1
=
=
B
1
<
<
*
!
C
B
C
B
+
1
B
+
!
;
B
*
+
1
H
;
<
A
w
+
1
!
+
B
C
+
1
*
+
;
1
x
'
y
?
&
+
1
B
;
B
+
B
C
+
1
<
*
A
w
!
x
@
A
y
A
&
+
1
2
B
1
!
=
E
+
!
C
!
!
+
B
x
'
B
y
C
<
+
1
ƒ
!
A
*
!
=
<
C
C
*
+
x
ƒ
y
C
!
+
1
A
*
|
*
+
+
+
1
3
4
5
/
6
/
-
/
.
/
/
+
B
!
+
B
/
+
1
.
/
!
B
0
.
/
C
3
B
.
;
:
.
3
4
.
+
2
-
.
1
-
0
+
-
1
!
=
+
!
<
1
+
+
!
<
C
;
B
1
!
B
w
;
1
B
B
;
!
B
<
+
w
A
+
!
!
C
B
@
+
1
*
<
<
+
1
B
=
B
1
!
C
B
!
!
B
‚
!
*
‚
*
=
B
w
!
+
1
w
=
'
=
B
&
C
+
1
<
<
+
!
1
;
!
U
C
+
B
1
B
!
H
=
B
E
<
+
+
!
A
!
w
C
+
!
1
0
1
2
›
/
/
4
/
5
0
0
B
+
!
+
!
C
!
|
+
B
C
+
1
!
<
U
E
;
!
A
+
+
1
B
+
!
<
+
!
C
B
š
J
M
3
The EIS spectra by this Randle’s equivalent circuit were recorded for every step of the gold SPE
6
-
›
0
0
*
!
H
0
0
1
0
1
1
1
1
-
C
B
+
<
+
1
!
*
+
H
!
;
!
+
<
0
w
‚
*
+
;
+
š
=
K
(
1
=
<
3
/
:
B
+
<
+
1
/
z
E
7
7
{
A
!
<
;
w
<
1
=
1
<
B
+
!
+
!
C
!
!
+
B
<
*
+
1
/
z
E
7
7
{
w
!
+
<
+
1
=
<
1
A
1
@
*
!
H
!
w
U
;
B
+
<
&
H
=
+
1
A
B
9
H
|
B
+
!
+
+
B
+
!
B
+
A
+
H
+
1
*
B
1
!
=
<
B
!
A
U
w
B
B
<
=
!
*
;
x
E
7
7
{
y
C
+
1
;
w
!
B
w
!
<
+
1
=
+
@
w
B
1
!
=
<
!
<
U
;
!
A
6
+
H
|
w
+
1
+
+
1
/
z
A
B
|
A
C
+
1
;
w
!
C
B
+
<
.
/
1
1
|
B
+
@
+
*
C
+
+
=
1
B
w
!
!
A
&
+
U
w
1
*
!
=
!
<
*
*
B
;
;
=
!
+
<
1
*
B
<
B
+
!
B
*
+
!
+
!
C
+
!
!
B
!
+
!
+
<
1
(
+
*
*
1
!
C
B
1
H
C
!
*
A
<
‚
*
*
+
!
+
2
3
4
1
6
1
<
5
0
1
4
1
1
3
0
B
2
B
0
/
0
0
C
.
*
!
C
B
B
+
<
!
w
+
+
1
;
!
@
*
w
+
<
*
+
!
B
!
A
U
w
B
C
*
B
+
O
+
1
A
B
C
5
2
6
2
-
2
.
2
/
2
0
2
1
l
B
+
!
+
+
B
+
!
B
+
1
<
!
<
+
1
B
+
!
+
!
C
!
;
!
B
<
+
<
A
w
+
1
=
+
@
w
B
1
!
=
<
D
E
!
<
U
;
!
A
1
U
+
+
=
H
;
!
+
A
<
=
+
1
+
1
<
!
<
+
1
B
+
!
B
+
!
C
!
&
!
C
B
+
<
F
G
1
!
*
<
@
A
w
+
1
B
!
=
;
<
B
@
*
C
+
1
:
6
3
;
B
+
!
(
+
1
*
=
1
w
;
+
@
w
B
1
!
=
<
H
I
J
!
+
1
;
{
B
<
+
C
+
1
!
<
U
;
!
A
*
+
x
+
B
+
!
B
;
+
N
N
y
&
+
D
<
;
B
|
=
K
L
D
M
D
D
D
E
D
F
D
;
D
w
1
!
D
*
!
+
C
B
!
*
B
+
+
1
&
;
@
!
B
<
*
B
+
!
=
A
*
=
+
<
+
D
L
E
M
/
:
C
E
D
E
E
B
<
C
<
B
+
!
<
1
!
*
+
<
B
+
<
A
w
C
*
!
+
1
!
*
A
+
+
B
!
B
+
+
H
+
1
+
1
@
!
<
C
B
+
+
;
†
—
+
A
!
A
@
!
+
!
!
C
1
!
+
1
!
+
=
<
H
U
;
!
A
C
B
B
H
<
A
+
+
w
1
+
1
=
<
U
+
!
B
!
+
1
B
+
!
+
!
C
!
!
+
B
&
C
1
*
A
‚
*
+
B
!
B
1
!
=
+
!
C
!
!
+
+
Œ
;
†
ž
œ
Œ
†
Š
<
Ÿ
+
ž
+
1
Š
=
†
<
3
/
:
*
!
C
B
O
—
G
¸
·
¸
Ô
¸
Û
à
×
Ø
à
Ö
P
×
¾
¼
ß
ß
Í
¾
½
Û
H
I
E
F
Ô
E
<
'
E
<
J
K
E
1
I
D
E
+
H
!
D
+
G
3
D
!
z
w
!
+
+
@
:
6
3
A
*
+
w
!
@
<
<
+
B
C
!
+
C
+
1
B
1
B
J
E
K
E
L
F
M
F
D
F
E
F
F
<
C
B
+
+
!
<
*
B
<
=
<
*
!
C
B
7
@
!
&
+
1
!
*
+
A
+
<
*
;
;
!
+
<
+
1
;
!
@
*
›
F
F
F
!
B
!
L
+
H
H
H
H
H
+
A
<
+
1
+
1
B
+
+
*
<
!
+
!
š
C
=
K
!
;
5
!
B
1
<
*
;
;
+
B
+
1
+
C
/
B
z
*
!
!
E
7
+
7
{
+
+
=
w
<
<
!
+
1
*
1
+
=
<
1
;
|
E
+
!
E
;
|
;
!
+
C
+
w
;
B
!
!
<
U
;
!
A
@
!
B
(
*
*
!
C
B
(
+
1
*
A
‚
*
+
D
+
+
;
+
1
/
z
E
7
7
{
C
<
B
!
<
!
*
<
+
1
<
B
9
B
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